期刊
ORGANIC LETTERS
卷 10, 期 18, 页码 3945-3947出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol801500b
关键词
-
资金
- EPSRC
- European Comission [MEIF-CT-2006-041629]
Synthesis of beta,meso,beta-anthracene triply fused and beta,meso-anthracene doubly fused porphyrins has been achieved via oxidative intramolecular ring closure of meso-(9-anthryl)porphyrins and meso-(1-anthryl)porphyrins, respectively. Fusion was only possible when the anthracene carried electron-donating alkoxy substituents. The fused porphyrins exhibit strongly red-shifted UV-vis absorption spectra and reduced electrochemical HOMO-LUMO gaps (relative to the unfused tetraaryl porphyrin precursor).
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