期刊
ORGANIC LETTERS
卷 10, 期 18, 页码 4101-4104出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol801665z
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资金
- National Natural Science Foundation of China [20672126, 20721003]
- Chinese Academy of Sciences
- Shanghai Rising-Star Program [08QH 14027]
- Major State Basic Research Development Program [2006CB806106]
The first Rh-diene-catalyzed aqueous asymmetric 1,4-addition of alpha,6-unsaturated carbonyl compounds with arylboronic acids has been realized. By using a hydrophilic bicyclo[3.3.0] diene ligand, the reactions can be performed successfully in neat water at room temperature to afford the corresponding products in good yields and with very high enantioselectivities for both cyclic and linear substrates.
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