期刊
ORGANIC LETTERS
卷 10, 期 23, 页码 5321-5324出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol8016148
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资金
- Fonds der Chemischen Industrie
- Catalysts and Catalytic Reactions for Organic Synthesis [GRK 1038]
Rapid access to highly functionalized alkylidene cyclohexanols through a one-pot desymmetrizing hydroformylation/carbonyl ene cyclization starting from simple bisalkenylcarbinols is reported. Mechanistic insight into the carbonyl ene reaction is given, highlighting the importance of hyperconjugative substituent effects.
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