期刊
ORGANIC LETTERS
卷 10, 期 17, 页码 3817-3820出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol801502h
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资金
- National Science Foundation [CHE-0449587]
- NIH [GM-079339]
- Packard Foundation
- Beckman Foundation
- Sloan Foundation
- Cottrell Scholar
alpha-Chloroaldehyde bisulfite adducts were successfully employed in chiral NHC-catalyzed hetero-Diels-Alder reactions with various oxodienes under biphasic reaction conditions with high levels of enantioselectivity. This new protocol makes possible entantioselective additions from commercially available chloroacetaldehyde sodium bisulfite and demonstrates that this unique class of catalysts readily tolerates aqueous conditions.
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