期刊
ORGANIC & BIOMOLECULAR CHEMISTRY
卷 12, 期 18, 页码 2895-2902出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c3ob42470g
关键词
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资金
- Chinese National Natural Science Foundation [21202135]
- Natural Science Foundation of Fujian Province of China [2013J05031]
- NFFTBS [J1210014]
- National Basic Research Program of China [2012CB821600]
We present a novel and highly efficient methodology that allows for the construction of C-P bonds via the palladium-catalyzed air-based oxidative coupling of various commercially available arylboronic acids with easily oxidized H-phosphine oxides leading to valuable aryl phosphine oxides, particularly triarylphosphine oxides, with the use of air as the green oxidant, broad substrate applicability and good to excellent yields. The described catalytic system should be an efficient complement to the Chan-Lam type reaction and be useful in synthetic programs.
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