期刊
ORGANIC & BIOMOLECULAR CHEMISTRY
卷 11, 期 39, 页码 6691-6694出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c3ob41424h
关键词
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资金
- Natural Science Foundation of China [21172205, 21272222, 20972144, 91213303, 20932002, 31070211, J1030412]
- Ministry of Science and Technology of China [2010CB912103]
A cobalt-catalyzed oxidative [3 + 2] cycloaddition cascades of dihydroisoquinoline esters with nitroolefins or N-sulfuryl aldimines were developed at room temperature. A multi-component reaction for the synthesis of 5,6-dihydroimidazo[2,1-a]isoquinolines were also realized under almost identical conditions. This method is particularly suitable for the synthesis of tricyclic nitrogen heterocycles due to its simple manipulation, wide scope of the reaction substrates and excellent regioselectivity.
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