期刊
ORGANIC & BIOMOLECULAR CHEMISTRY
卷 10, 期 38, 页码 7681-7684出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c2ob26247a
关键词
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资金
- FAPESP [09/07281-0]
- CNPq (INCT-Catalise)
- CNPq (INBEQMeDI)
- Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP) [09/07281-0] Funding Source: FAPESP
An eco-friendly synthesis of highly functionalized epoxides and their incorporation into an organocatalytic multicomponent approach are reported. For this, a modified class of diarylprolinol silyl ethers was designed to enable high catalytic activity in an environmentally benign solvent system. The one-pot procedure showed great efficiency in promoting stereoselective multicomponent transformations in a tandem, 'green' fashion. Because of its non-residual, efficient and selective character, this synthetic design shows promise for large-scale applications in both diversity and target-oriented syntheses.
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