期刊
OPTICS LETTERS
卷 33, 期 21, 页码 2533-2535出版社
OPTICAL SOC AMER
DOI: 10.1364/OL.33.002533
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资金
- ACS Petroleum Research Fund
- National Science Foundation (NSF)
- Division Of Chemistry
- Direct For Mathematical & Physical Scien [748501] Funding Source: National Science Foundation
We present what we believe to be the first implementation of nonequilibrium two-dimensional IR spectroscopy (2DIR) combining electronic excitation within the Fourier transform (FT) approach. Nonequilibrium 2DIR spectra of Mn-2(CO)(10) and its photoproducts are obtained in two modalities: photoexcitation at 400 nm, either before a 2DIR probe or during the waiting time of the FT 2DIR measurement. Extending FT 2DIR to nonequilibrium systems offers insight into complex condensed-phase reaction dynamics. (D 2008 Optical Society of America
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