期刊
OPTICS EXPRESS
卷 22, 期 9, 页码 A867-A879出版社
OPTICAL SOC AMER
DOI: 10.1364/OE.22.00A867
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资金
- International Collaborative R&D Program - Korean Ministry of Knowledge Economy
- Korea Institute for Advancement of Technology (KIAT), Golbal Research Network program [2011-220-D00064]
- Basic Science Research Program through the National Research Foundation of Korea (NRF) - Ministry of Education, Science and Technology [2009-0094036]
Photo-electrodes with tailored three-dimensional nanostructures offer a large enhancement in light harvesting capability for various optoelectronic devices enabled by strong light scattering in the nanostructures as well as improved charge transport. Here we present an array of three-dimensional titanium dioxide (TiO2) nanohelixes fabricated by the oblique angle deposition method as a multifunctional photoanode for CdSe quantum dot sensitized solar cells (QDSSCs). The CdSe QDSSC with a TiO2 nanohelix photoanode shows a 100% higher power conversion efficiency despite less light being absorbed in CdSe QDs when compared with a conventional TiO2 nanoparticle photoanode. We attribute the higher power conversion efficiency to strong light scattering by the TiO2 nanohelixes and much enhanced transport and collection of photo-generated carriers enabled by the unique geometry and near-single crystallinity of the TiO2 nanohelix structure. (C)2014 Optical Society of America
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