期刊
NEW JOURNAL OF CHEMISTRY
卷 35, 期 12, 页码 2766-2772出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c1nj20516a
关键词
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资金
- Ministerio de Ciencia e Innovacion (MICINN)
- Ministerio de Educacion (MEC) of Spain [CTQ2010-20387, CTQ2009-07881/BQU, CTQ2007-62771/BQU]
- Consolider Ingenio [CSD2007-00006]
- FEDER
- Generalitat de Catalunya [SGR2009-01441]
- Agence Nationale de la Recherche [CP2D-MESORCAT]
- Generalitat Valenciana [GV/2007/142, PROMETEO/2009/039]
- University of Alicante
A new organic-inorganic hybrid silica material derived from a bis-silylated prolinamide by sol-gel methodology has been successfully applied as a supported organocatalyst in asymmetric aldol and Michael reactions. Our immobilized system presents similar performances to homogeneous prolinamides and added advantages of easy recovery and good recyclability. It fits green chemistry requirements as the reactions are performed in water, at room temperature, with low catalyst loadings (2-16 mol%).
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