期刊
NEW JOURNAL OF CHEMISTRY
卷 34, 期 4, 页码 714-717出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/b9nj00732f
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资金
- Ministry of Education, Culture, Sports, Science and Technology, Japan (MEXT) [19760536]
Molecularly imprinted polymers containing a photosensitizer, rose bengal (RB), were synthesized via a polymerization of methacrylic acid (MAA) as a functional monomer and chlorophenols as template molecules. The polymeric sensitizers promote selective oxidation of target chlorophenol in water with molecular oxygen under visible light irradiation (lambda > 530 nm). This is due to the selective attraction of the target substrate onto the molecular recognition site on the polymer followed by efficient oxidation of the substrate by a singlet oxygen produced by the photoexcited RB units located in the vicinity of the recognition site.
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