期刊
NATURE PHOTONICS
卷 6, 期 2, 页码 115-120出版社
NATURE PUBLISHING GROUP
DOI: 10.1038/NPHOTON.2011.317
关键词
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资金
- Office of Naval Research [N000141110245]
- Department of Energy Basic Energy Sciences [DE-FG0207ER46464]
- Air Force Office of Scientific Research [FA9550-09-1-0320]
Inverted polymer bulk heterojunction solar cells have received a great deal of attention because of their compatibility with large-scale roll-to-roll processing. The inverted cell geometry has the following structure: substrate (rigid or flexible)/indium tin oxide/electron-transporting layer/photoactive layer/hole-transporting layer/top anode. Solution-processed metal-oxide films, based on materials such as ZnO and TiO2, are typically used as the electron-transporting layers. Here, we demonstrate enhanced charge collection in inverted polymer solar cells using a surface-modified ZnO-polymer nanocomposite electron-transporting layer. Using this approach, we demonstrate inverted polymer solar cells based on a low-bandgap polymer with an alternating dithienogermole-thienopyrrolodione repeat unit (PDTG-TPD) with certified power conversion efficiencies of 7.4%. To our knowledge, this is the highest efficiency reported to date for polymer solar cells with a device architecture compatible with the roll-to-roll process.
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