4.8 Article

Quantum criticality in a metallic spin liquid

期刊

NATURE MATERIALS
卷 13, 期 4, 页码 356-359

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NATURE PUBLISHING GROUP
DOI: 10.1038/NMAT3900

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资金

  1. German Science Foundation [FOR 960]
  2. Helmholtz Virtual Institute [VH521]
  3. JSPS [25707030]
  4. PRESTO of JST
  5. National Science Foundation [PHYS-1066293]
  6. hospitality of the Aspen Center for Physics
  7. Grants-in-Aid for Scientific Research [25707030, 14F04026] Funding Source: KAKEN

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When magnetic order is suppressed by frustrated interactions, spins form a highly correlated fluctuating 'spin liquid' state down to low temperatures. The magnetic order of local moments can also be suppressed when they are fully screened by conduction electrons through the Kondo effect. Thus, the combination of strong geometrical frustration and Kondo screening may lead to novel types of quantum phase transition. We report low-temperature thermodynamic measurements on the frustrated Kondo lattice Pr2Ir2O7, which exhibits a chiral spin liquid state below 1.5 K as a result of the frustrated interaction between Ising 4f local moments and their interplay with Ir conduction electrons. Our results provide a first clear example of zero-field quantum critical scaling that emerges in a spin liquid state of a highly frustrated metal.

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