期刊
NANOSCALE
卷 5, 期 3, 页码 1188-1194出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c2nr33114d
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资金
- National Research Foundation of Korea (NRF) [R15-2008-006-03002-0]
- World Class University Program (WCU) at GIST [R31-2008-000-10026-0]
- Ministry of Education, Science and Technology (MEST)
- GSR-IC project at GIST
- National Research Foundation of Korea (NRF, CLEA, NCRC) [2011-0029414]
- Ministry of Education, Science & Technology (MoST), Republic of Korea [gist-03-06] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)
- Ministry of Science, ICT & Future Planning, Republic of Korea [GIST-03-06] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)
- National Research Foundation of Korea [R15-2008-006-03002-0, 2011-0029414] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)
One-dimensional (1-D) SnO2 nanorods (NRs) with a rutile structure are grown on various substrates regardless of the lattice-mismatch by using a new nutrient solution based on tin oxalate, which generated supersaturated Sn2+ sources. These affluent sources are appropriate for producing a large number of SnO2 nanoparticles, sufficient for stacking on a substrate surface by gravity, which then acts as a seed layer for subsequent nanorod growth. Single crystalline nanorods are grown along the [001] direction by the oriented attachment phenomenon in which the attached nanoparticles were rearranged to reduce the overall surface energy through sharing thermodynamically unstable crystal (001) planes. Furthermore, the grown SnO2 NRs are covered with a TiO2 particulate film and utilized as a photoanode in DSSCs. The power conversion efficiency is 8.61%, enhanced by 14.2% compared to the photoanode with only a TiO2 particulate film.
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