4.8 Article

Nanoscale Fluorescence Lifetime Imaging of an Optical Antenna with a Single Diamond NV Center

期刊

NANO LETTERS
卷 13, 期 8, 页码 3807-3811

出版社

AMER CHEMICAL SOC
DOI: 10.1021/nl401791v

关键词

Near-field scanning optical microscopy; NV center; fluorescence lifetime imaging; local density of optical states; optical antenna

资金

  1. Department of Energy [DE- FG02-05ER46207]
  2. Office of Naval Research Young Investigator Award [N00014-11-1-0645]
  3. DARPA Young Faculty Award
  4. Physics Division, U.S, Army Research Office
  5. [W911NF0910425]

向作者/读者索取更多资源

Solid-state quantum emitters, such as artificially engineered quantum dots or naturally occurring defects in solids, are being investigated for applications ranging from quantum information science and optoelectronics to biomedical imaging. Recently, these same systems have also been studied from the perspective of nanoscale metrology. In this letter, we study the near-field optical properties of a diamond nanocrystal hosting a single nitrogen vacancy center. We find that the nitrogen vacancy center is a sensitive probe of the surrounding electromagnetic mode structure. We exploit this sensitivity to demonstrate nanoscale fluorescence lifetime imaging microscopy (FLIM) with a single nitrogen vacancy center by imaging the local density of states of an optical antenna.

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