4.8 Article

Plasmonic Nature of the Terahertz Conductivity Peak in Single-Wall Carbon Nanotubes

期刊

NANO LETTERS
卷 13, 期 12, 页码 5991-5996

出版社

AMER CHEMICAL SOC
DOI: 10.1021/nl403175g

关键词

Single-wall carbon nanotubes; terahertz; plasmon resonance; density gradient ultracentrifugation

资金

  1. Department of Energy [DE-FG02-06ER46308]
  2. National Science Foundation [OISE-0530220, EEC-0540832]
  3. Robert A. Welch Foundation [C-1509]

向作者/读者索取更多资源

Plasmon resonance is expected to occur in metallic and doped semiconducting carbon nanotubes in the terahertz frequency range, but its convincing identification has so far been elusive. The origin of the terahertz conductivity peak commonly observed for carbon nanotube ensembles remains controversial. Here we present results of optical, terahertz, and direct current (DC) transport measurements on highly enriched metallic and semiconducting nanotube films. A broad and strong terahertz conductivity peak appears in both types of films, whose behaviors are consistent with the plasmon resonance explanation, firmly ruling out other alternative explanations such as absorption due to curvature-induced gaps.

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