4.8 Article

Strong Enhancement of Light-Matter Interaction in Graphene Coupled to a Photonic Crystal Nanocavity

期刊

NANO LETTERS
卷 12, 期 11, 页码 5626-5631

出版社

AMER CHEMICAL SOC
DOI: 10.1021/nl302746n

关键词

Graphene; photonic crystal cavity; optoelectronics; Raman spectroscopy

资金

  1. Air Force Office of Scientific Research PECASE
  2. DARPA Information in a Photon program [W911NF-10-1-0416]
  3. National Science Foundation [DMR-1106225]
  4. U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886]
  5. Center for Re-Defining Photovoltaic Efficiency Through Molecule Scale Control, an Energy Frontier Research Center
  6. U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001085]
  7. Division Of Materials Research
  8. Direct For Mathematical & Physical Scien [1106225] Funding Source: National Science Foundation

向作者/读者索取更多资源

We demonstrate a large enhancement in the interaction of light with graphene through coupling with localized modes in a photonic crystal nanocavity. Spectroscopic studies show that a single atomic layer of graphene reduces the cavity reflection by more than a factor of one hundred, while also sharply reducing the cavity quality factor. The strong interaction allows for cavity-enhanced Raman spectroscopy on subwavelength regions of a graphene sample. A coupled mode theory model matches experimental observations and indicates significantly increased light absorption in the graphene layer. The coupled graphene cavity system also enables precise measurements of graphene's complex refractive index.

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