期刊
NANO LETTERS
卷 11, 期 2, 页码 767-771出版社
AMER CHEMICAL SOC
DOI: 10.1021/nl103977d
关键词
Graphene; electrical properties; thermal annealing; wet-chemical treatment; sensor
类别
资金
- Foundation of CAS [KJCX2.YW.M15]
- 973 Fund [2011CB932700]
- National Natural Science Foundation of China [20973045]
By combining atomic force microscopy and transport measurements, we systematically investigated effects of thermal annealing on surface morphologies and electrical properties of single-layer graphene devices fabricated by electron beam lithography on silicon oxide (SiO2) substrates. Thermal treatment above 300 degrees C in vacuum was required to effectively remove resist residues on graphene surfaces. However, annealing at high temperature was found to concomitantly bring graphene in close contact with SiO2 substrates and induce increased coupling between them, which leads to heavy hole doping and severe degradation of mobilities in graphene devices. To address this problem, a wet-chemical approach employing chloroform was developed in our study, which was shown to enable both intrinsic surfaces and enhanced electrical properties of graphene devices. Upon the recovery of intrinsic surfaces of graphene, the adsorption and assisted fibrillation of amyloid beta-peptide (A beta-42) on graphene were electrically measured in real time.
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