期刊
NANO LETTERS
卷 10, 期 8, 页码 3062-3067出版社
AMER CHEMICAL SOC
DOI: 10.1021/nl101605r
关键词
Coherent phonons; quantum dots; piezoelectricity; femtosecond spectroscopy
类别
资金
- CFI
- NSERC
- FQRNT
- McGill University
- Max Binz
By direct observation of coherent acoustic phonons, we demonstrate a novel extrinsic piezoelectric response in colloidal CdSe semiconductor quantum dots. This response is driven by the migration of charges to the surface of the quantum dot on a vibrationally impulsive time scale. Surface- and fluence-dependent studies reveal that the observed carrier capture based piezo response is controllable and is at least an order of magnitude larger titan the intrinsic piezo response of wurtzite CdSe.
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