期刊
NANO LETTERS
卷 10, 期 7, 页码 2381-2386出版社
AMER CHEMICAL SOC
DOI: 10.1021/nl100343j
关键词
Single-walled carbon nanotubes; ultrafast optical spectroscopy; multiple exciton generation; carrier multiplication; excited-state dynamics
类别
资金
- US Department of Energy Office of Basic Energy Sciences
Upon absorption of single photons, multiple excitons were generated and detected in semiconducting single-walled carbon nanotubes (SWNTs) using transient absorption spectroscopy For (6,5) SWNTs, absorption of single photons with energies corresponding to three times the SWNT energy gap results in an exciton generation efficiency of 130% per photon Our results suggest that the multiple exciton generation threshold in SWNTs can be close to the limit defined by energy conservation
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