期刊
MOLECULAR PHYSICS
卷 112, 期 9-10, 页码 1257-1261出版社
TAYLOR & FRANCIS LTD
DOI: 10.1080/00268976.2014.889325
关键词
statistical thermodynamics; nanoporous materials; structural transitions; adsorption
资金
- Agence Nationale de la Recherche under project 'SOFT-CRYSTAB' [ANR-2010-BLAN-0822]
We briefly review the concept of temperature-loading phase diagram that we derived from an osmotic statistical ensemble analysis of the adsorption-induced structural transitions observed in the MIL-53 family of metal-organic framework nanoporous materials. We highlight the generic nature of this diagram and comment on the occurrence of breathing transitions depending on the guest fluid, the framework functionalisation and the nature of the metal centre.
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