期刊
MOLECULAR PHYSICS
卷 110, 期 21-22, 页码 2781-2796出版社
TAYLOR & FRANCIS LTD
DOI: 10.1080/00268976.2012.705347
关键词
van der Waals complexes; acetylene; overtone spectroscopy; supersonic expansion; cavity ring-down spectroscopy
资金
- EU
- ULB
- FRS-FNRS
- Federation Wallonie-Bruxelles (ARC project)
Spectroscopic results are presented concerning the 2CH excitation around 1.5 mu m in van der Waals complexes of acetylene (C2H2) with Ar, Kr, N-2, CO2, N2O and C2H2. Many are reviewed from the literature, with some updates. Previously unpublished results are also presented, concerning the mechanism of formation of C2H2-Ar in the supersonic jet, the assignment of new spectral structures in C2H2-N2O, and the first observation of 2CH excitation in C2H2-Ne, C2H2-H2O, C2H2-D2O and (C2H2)(n). Lifetimes of these 2CH vibrationally excited dimers are discussed.
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