期刊
MOLECULAR PHYSICS
卷 108, 期 11, 页码 1415-1433出版社
TAYLOR & FRANCIS LTD
DOI: 10.1080/00268971003762134
关键词
x-ray and neutron scattering; x-ray absorption and emission spectroscopy; mixture and continuum models; empirical and ab initio theory
资金
- NSF
- Department of Energy
We review the spectroscopic techniques and scattering experiments used to probe the structure of water, and their interpretation using empirical and ab initio models, over the last 5 years. We show that all available scientific evidence overwhelmingly favors the view of classifying water near ambient conditions as a uniform, continuous tetrahedral liquid. While there are controversial issues in our understanding of water in the supercooled state, in confinement, at interfaces, or in solution, there is no real controversy in what is understood as regards bulk liquid water under ambient conditions.
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