期刊
MICROPOROUS AND MESOPOROUS MATERIALS
卷 142, 期 1, 页码 276-281出版社
ELSEVIER
DOI: 10.1016/j.micromeso.2010.12.010
关键词
Titania; Photocatalysis; Carbon-doping; Mesoporous film
类别
资金
- National Science Foundation of China [30670522]
- Hi-Tech Research and Development Program (863 Program) of China [2006AA10Z436]
- Social Developing Program of Jiangsu Province [BE2008643]
A visible-light-active C-doped mesoporous TiO2 film was prepared by sol-gel process combined with hydrothermal treatment. Glucose was used as carbon source and structure-directing agent. The structure and physicochemical properties of the film were characterized by X-ray diffraction (XRD), N-2 adsorption-desorption isotherms, scanning electron microscopy (SEM), Fourier transform-infrared spectroscopy (FT-IR), X-ray photoelectron spectroscopy (XPS), UV-vis diffuse reflectance spectrum (DRS) and photoluminescence (PL). The results indicated that oxygen sites in the TiO2 lattice were substituted by carbon atoms and an O-Ti-C bond was formed. The C-doped mesoporous TiO2 film had a high surface area of 283 m(2) g(-1). The film was about 10 mu m thick and was composed of anatase TiO2 particles. The prepared C-doped TiO2 film exhibited excellent photocatalytic activity in the degradation of dye Reactive Brilliant Red X-3B (C.I. reactive red 2) under UV and visible light irradiation compared with that of the smooth TiO2 film and P25 film. The recycle ability of the C-doped mesoporous TiO2 film was also investigated. The degradation ratio which was still higher than 87% after 5 cycles, decreased by 3% compared to the first cycle. (C) 2010 Elsevier Inc. All rights reserved.
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