期刊
MICROPOROUS AND MESOPOROUS MATERIALS
卷 141, 期 1-3, 页码 231-235出版社
ELSEVIER SCIENCE BV
DOI: 10.1016/j.micromeso.2010.10.048
关键词
Lithium doping; Carbon dioxide (CO2); Metal-organic framework (MOF); Separation; Adsorption
类别
资金
- U.S. Department of Energy [DE-FG02-08ER15967]
- Northwestern NSEC
- U.S. Department of Energy (DOE) [DE-FG02-08ER15967] Funding Source: U.S. Department of Energy (DOE)
Incorporation of Li cations into MOFs by either of two methods, chemical reduction or cation exchange, significantly improves the CO2/CH4 selectivity. While the selectivity enhancement by the chemical reduction seems to come from favorable displacement of catenated frameworks, the selectivity improvement by the Li cation exchange comes from enhanced solid-gas interactions. (C) 2010 Elsevier Inc. All rights reserved.
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