期刊
APPLIED SURFACE SCIENCE
卷 356, 期 -, 页码 1341-1348出版社
ELSEVIER SCIENCE BV
DOI: 10.1016/j.apsusc.2015.08.079
关键词
Photocatalyst; BiOCl; Structure; Visible light
类别
资金
- National Natural Science Foundation of China [Y3J1391A21, 51372267, 51210105026, 51172270]
- National Basic Research Program of China [2013CB932901]
- Chinese Academy of Sciences
Through the incorporation of Pb2+ into the [Bi2O2] layers, the BiPbO2Cl nanosheets with layered structure have been successfully synthesized by one-step solvothermal method. The lattice parameters of tetragonal BiPbO2Cl are a = 3.9417(2) angstrom and c= 12.3957(6) angstrom, where the c value is considerably smaller than previous results. The structure of BiPbO2Cl was then readdressed through Rietveld refinement and aberration-corrected scanning transmission electron microscope investigations. The photo-decomposition experiments demonstrated that BiPbO2Cl nanosheet exhibits high photocatalytic activity, which is 12.6 times higher than that of BiPbO2Cl bulk. The photocurrent measurement suggests a more efficient photoinduced charge separation and transfer in BiPbO2Cl nanosheet. (C) 2015 Elsevier B.V. All rights reserved.
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