期刊
MACROMOLECULES
卷 45, 期 17, 页码 7163-7170出版社
AMER CHEMICAL SOC
DOI: 10.1021/ma301337e
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资金
- Air Force Office of Scientific Research
- Materials and Manufacturing Directorate of the Air Force Research Laboratory
The potential for wireless transduction of input light energy into mechanical outputs has led to a reinvigorated pursuit of photomechanical effects in polymeric materials and composites. We report here on factors influencing the photochemical mechanism (and thus the mechanical output) in monodomain azobenzene-functionalized liquid crystal polymer networks. Through systematic examination of a representative material with both mechanics and spectroscopic characterization the prevalence of the trans-cis and trans-cis-trans mechanisms is elucidated. Furthermore, the role of light intensity in generating heat (photothermal effects) is also reported.
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