期刊
MACROMOLECULAR RAPID COMMUNICATIONS
卷 36, 期 7, 页码 610-615出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/marc.201400553
关键词
block copolymers; metal-ligand interaction; smart materials; supramolecular assembly
资金
- F.R.I.A.
At the basis of smart self-assembled materials are lying small building blocks that can hierarchically assemble in response to stimuli, e.g., temperature or chemical species. In this context, the synthesis of terpyridine end-capped poly(2-(dimethylamino)ethyl methacrylate)-block-poly(N-isopropylacrylamide) diblock copolymers via controlled radical copolymerization is reported here. The self-assembly of those copolymers is investigated in dilute aqueous solutions while varying temperature or adding transition metal ions, respectively, leading to the formation of micellar nanostructures or metallosupramolecular triblock copolymers.
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