Radon concentration in soil gas and its correlations with pedologies, permeabilities and 226Ra content in the soil of the Metropolitan Region of Belo Horizonte - RMBH, Brazil

The radon concentration in soil gas is directly dependent on the geological characteristics of the area, such as lithology, pedology and on geochemicals, physicals and mineralogicals parameters of the soil. This paper looks for correlations between radon concentrations in soil gas and its soil permeability, U-238, Th-232 and Ra-226 contents in the soil groups classified by pedologies of Metropolitan Region of Belo Horizonte (RMBH), Minas Gerais, Brazil. The soil gas radon concentrations were determined by using an A/phaGUARD monitor at about 150 measurement points. In soil samples of the same measurement points, the concentrations of Ra-226 were determined by gamma spectrometry (HPGe), and U-233 and Th-232 by ICP-MS. The soil permeabilities were determined by using the RADON-JOK (R) permeameter. The mean concentrations of radon in soil gas ranged from 13.6 +/- 3.0 kBq m(-3) for Litholic Neosols until 60.6 +/- 8.7 kBq m(-3) for Perferric Red Latosols. The mean of Ra-226 activity concentrations presented variation of 12.4 +/- 2.5 Bq kg(-1) for Litholic Neosols until 50.3 +/- 13 Bq kg(-1) for Perferric Red Latosols. Approximately 40% of the soils presented high permeability. The areas of different pedologies were classified by Soil Radon Index (SRI), determined by the soil gas radon concentration and permeability. Approximately 53% of the Perferric Red Latosols measurement site could be classified as High Risk (Swedish criteria). The preliminary results may indicate an influence of iron formations present very close to the Perferric Red Latosols in the retention of uranium minerals, and hence an increase in the concentration of radon and radium, whereas the series are in equilibrium in the environment. (C) 2015 Elsevier Ltd. All rights reserved.