期刊
LANGMUIR
卷 28, 期 2, 页码 1539-1544出版社
AMER CHEMICAL SOC
DOI: 10.1021/la203990n
关键词
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资金
- Japan Society for the Promotion of Science
- Grants-in-Aid for Scientific Research [11J03906] Funding Source: KAKEN
The nanointegration mechanism for photoinduced hydrogen nano-generators using nanogels is described. By spatially integrating poly(N-isopropylacrylamide-co-Ru(bpy)(3)) nanogels as a photosensitizer and Pt nanoparticles as a catalyst, a mechanism using electrostatic interactions and the shrinking behavior of the thermosensitive polymer network is revealed. In addition, to evaluate the sensitivity to exterior energy, light, and heat, the integrated nanospace is controlled by using thermosensitive nanogels, which drastically shrink above the volume phase transition temperature. Such nanospatial control of multiple kinds of functional molecules in a photochemical reaction, is important for the realization of artificial photosynthetic systems.
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