期刊
LANGMUIR
卷 25, 期 14, 页码 8268-8273出版社
AMER CHEMICAL SOC
DOI: 10.1021/la900472d
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资金
- Kyushu University
- JST-MOST International Cooperation
Carbon nanofibers containing a range of nitrogen contents of 1-10 atom % were directly synthesized by catalytic chemical vapor deposition over nickel-based catalysts at 350-600 degrees C using acetonitrile and acrylonitrile. The nitrogen content was controlled by careful choice of the reaction conditions. The N-doped carbon nanofibers showed herringbone structure with 20-60 nm diameter. X-ray photoelectron spectroscopy was applied to examine the chemical state of nitrogen in carbon nanofibers. Structural features of N-doped carbon nanofibers were examined in X-ray diffraction and electron microscopy. The mechanism for nitrogen including the structure of carbon nanofibers through the catalysis was discussed on the basis of the results.
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