期刊
JOURNAL OF THE OPTICAL SOCIETY OF AMERICA B-OPTICAL PHYSICS
卷 26, 期 9, 页码 1736-1745出版社
OPTICAL SOC AMER
DOI: 10.1364/JOSAB.26.001736
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资金
- Enterprise Ireland
- Science Foundation Ireland
- Basic Research and Research Frontiers Programmes
- Irish Research Council for Science, Engineering and Technology
The photochemical processes present during free-radical-based holographic grating formation are examined. A kinetic model is presented, which includes, in a more nearly complete and physically realistic way, most of the major photochemical and nonlocal photopolymerization-driven diffusion effects. These effects include: (i) non-steadystate kinetics (ii) spatially and temporally nonlocal polymer chain growth (iii) time varying photon absorption (iv) diffusion controlled viscosity effects (v) multiple termination mechanisms, and (vi) inhibition. The convergence of the predictions of the resulting model is then examined. Comparisons with experimental results are carried out in Part II of this series of papers [J. Opt. Soc. Am. B 26, 1746 (2009)]. (C) 2009 Optical Society of America
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