期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 140, 期 38, 页码 11931-11934出版社
AMER CHEMICAL SOC
DOI: 10.1021/jacs.8b08385
关键词
-
资金
- European Research Council [ERC AdG 692775]
- Planning and Budgeting Committee (PBC)
The synthesis of N-heteroaromatic compounds via an acceptorless dehydrogenative coupling process involving direct use of ammonia as the nitrogen source was explored. We report the synthesis of pyrazine derivatives from 1,2-diols and the synthesis of N substituted pyrroles by a multicomponent dehydrogenative coupling of 1,4-diols and primary alcohols with ammonia. The acridine-based Ru-pincer complex 1 is an effective catalyst for these transformations, in which the acridine backbone is converted to an anionic dearomatized PNP-pincer ligand framework.
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