期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 136, 期 25, 页码 8839-8842出版社
AMER CHEMICAL SOC
DOI: 10.1021/ja5044787
关键词
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资金
- 973 program [2013CB632402]
- NSFC [51272199, 51320105001, 51372190, 21177100]
Control of TiO2 crystal facets has attracted enormous interest due to the fascinating shape-dependent photocatalytic activity of this material. In this work, the effect of the ratio of {001} and {101} facets on the photocatalytic CO2-reduction performance of anatase TiO2 is reported. A new surface heterojunction concept is proposed on the basis of the density functional theory (DFT) calculations to explain the difference in the photocatalytic activity of TiO2 with coexposed {001} and {101} facets.
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