期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 136, 期 13, 页码 4829-4832出版社
AMER CHEMICAL SOC
DOI: 10.1021/ja5001888
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资金
- KAKENHI [22550098]
- Grants-in-Aid for Scientific Research [25105732, 22550098] Funding Source: KAKEN
Homogeneous perdehydrogenation of saturated bicyclic 2,6-dimethyldecahydro-1,5-naphthyridine and perhydrogenation of aromatic 2,6-dimethyl-1,5-naphthyridine with release and uptake of five molecules of H-2 are efficiently achieved by iridium complexes bearing a functional bipyridonate ligand. Successive perhydrogenation and perdehydrogenation of 2,6-dimethyl-1,5-naphthryridine using a single iridium complex also proceed with the reversible inter-conversion of the catalytic species, depending on the presence or absence of H-2.
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