期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 136, 期 4, 页码 1300-1303出版社
AMER CHEMICAL SOC
DOI: 10.1021/ja412342g
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资金
- NIH [GM104180]
- NSF GRFP [DGE-1346837]
- Italian Ministry for Education and Research
- Scripps Research Institute
- Eli Lilly
- Boehringer Ingelheim
- Amgen
- Baxter Foundation
Few methods permit the hydrogenation of alkenes to a thermodynamically favored configuration when steric effects dictate the alternative trajectory of hydrogen delivery. Dissolving metal reduction achieves this control, but with extremely low functional group tolerance. Here we demonstrate a catalytic hydrogenation of alkenes that affords the thermodynamic alkane products with remarkably broad functional group compatibility and rapid reaction rates at standard temperature and pressure.
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