期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 136, 期 4, 页码 1264-1267出版社
AMER CHEMICAL SOC
DOI: 10.1021/ja4117389
关键词
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资金
- 973 Program of China [2012CB626803]
- High Technology Research & Development Program of Xinjiang Uygur Autonomous Region of China [201315103, 201116143]
- National Natural Science Foundation of China [U1129301, 21201176, 51172277]
- Western Light Foundation Program of CAS [XBBS201214]
- Main Direction Program of Knowledge Innovation of CAS [KJCX2-EW-H03-03]
- National Science Foundation [DMR-1005827]
- ACS PRF [52138-DNI10]
Nonlinear optical (NLO) crystals are essential materials for generation of coherent UV light in solid state lasers. KBBF is the only material that can achieve coherent light below 200 nm by direct second harmonic generation (SHG). However, its strong layer habits and the high toxicity of the beryllium oxide powders required for synthesis limit its application. By substituting Be with Zn and connecting adjacent [Zn2BO3O2](infinity) layers by B3O6 groups, a new UV nonlinear optical material, Cs3Zn6B9O21, was synthesized. It overcomes the processing limitations of KBBF and exhibits the largest SHG response in the KBBF family.
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