期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 136, 期 36, 页码 12588-12591出版社
AMER CHEMICAL SOC
DOI: 10.1021/ja507167k
关键词
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资金
- Norman Hackerman Texas Advanced Research Program [003644-0060]
- NSF [CHE-0847736]
- HHMI grant, through the Undergraduate Science Education Program
- Direct For Mathematical & Physical Scien
- Division Of Chemistry [0847736] Funding Source: National Science Foundation
Here we report the synthesis of metalated main-chain polypseudorotaxanes via ring-opening olefin metathesis copolymerization of macrocycles and metalated [2]catenanes. By varying the feed ratio of the macrocycle and the [2]catenate comonomers, we prepared metalated pseudorotaxane polymers with selected, predictable average linear densities of threaded macrocycles that ranged from 0% to 100%, thus allowing, for the first time, both full and fine control over this key parameter.
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