期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 135, 期 33, 页码 12204-12207出版社
AMER CHEMICAL SOC
DOI: 10.1021/ja406338r
关键词
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资金
- Alexander von Humboldt Foundation
- European Research Council under the European Community/ERC [25936]
- DFG
Multisubstituted isoquinoline and pyridine N-oxides have been prepared by Rh(III)-catalyzed cyclization of oximes and diazo compounds via aryl and vinylic C-H activation. This intermolecular annulation involving tandem C-H activation, cyclization, and condensation steps proceeds under mild conditions, obviates the need for oxidants, releases N-2 and H2O as the byproducts, and displays a broad substituent scope.
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