期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 135, 期 13, 页码 4954-4957出版社
AMER CHEMICAL SOC
DOI: 10.1021/ja401061m
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资金
- Swedish Research Council (VR)
- Leverhulme Trust Early Career Research Fellowship
- ERC Advanced Grant
- EPSRC
- Royal Society Wolfson Merit award
- EPSRC [EP/I011870/1, EP/K038869/1, EP/K031082/1] Funding Source: UKRI
- Engineering and Physical Sciences Research Council [EP/K038869/1, EP/I011870/1, EP/K031082/1] Funding Source: researchfish
Porous NOTT-202a shows exceptionally high uptake of SO2, 13.6 mmol g(-1) (87.0 wt %) at 268 K and 1.0 bar, representing the highest value reported to date for a framework material. NOTT-202a undergoes a distinct irreversible framework phase transition upon SO2 uptake at 268-283 K to give NOTT-202b which has enhanced stability due to the formation of strong pi...pi interactions between interpenetrated networks.
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