期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 134, 期 35, 页码 14322-14325出版社
AMER CHEMICAL SOC
DOI: 10.1021/ja3065446
关键词
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资金
- Spanish MINECO [SAF2010-20822-C02, CTQ2010-15297, CTQ2010-14974, CSD2007-00006]
- ERDF
- Xunta de Galicia [INCITE09209084PR, GRC2010/12]
- Junta de Andalucia [2008/FQM-3833, 2009/FQM-4537]
- Fundacao para a Ciencia e Tecnologia (FCT, Portugal)
- POPH/FSE [SFRH/BD/60214/2009]
- Fundação para a Ciência e a Tecnologia [SFRH/BD/60214/2009] Funding Source: FCT
The first highly enantioselective intermolecular (4 + 2) cydoaddition between allenes and dienes is reported. The reaction provides good yields of optically active cyclohexenes featuring diverse substitution patterns and up to three stereocenters. Key to the success of the process is the use of newly designed axially chiral N-heterocyclic carbene-gold catalysts.
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