期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 134, 期 26, 页码 10773-10776出版社
AMER CHEMICAL SOC
DOI: 10.1021/ja3039807
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资金
- EPSRC
- ERC
- BBSRC
- Marie Curie Foundation
- Deutsche Forschungsgemeinschaft
- AstraZeneca
- Engineering and Physical Sciences Research Council [EP/I00548X/1] Funding Source: researchfish
- EPSRC [EP/I00548X/1] Funding Source: UKRI
Alkenes and arenes represent two classes of feedstock compounds whose union has fundamental importance to synthetic organic chemistry. We report a new approach to alkene arylation using diaryliodonium salts and Cu catalysis. Using a range of simple alkenes, we have shown that the product outcomes differ significantly from those commonly obtained by the Heck reaction. We have used these insights to develop a number of new tandem and cascade reactions that transform readily available alkenes into complex arylated products that may have broad. applications in chemical synthesis.
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