期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 134, 期 26, 页码 10942-10946出版社
AMER CHEMICAL SOC
DOI: 10.1021/ja303023n
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资金
- National Institutes of Health [GM099142]
The tandem ylide formation/[2,3]-sigmatropic rearrangement between donor/acceptor rhodium carbenoids and chiral allyl alcohols is a convergent C-C bond forming process, which generates two vicinal stereogenic centers. Any of the four possible stereoisomers can be selectively synthesized by appropriate combination of the chiral catalyst Rh-2(DOSP)(4) and the chiral alcohol.
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