期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 134, 期 4, 页码 2325-2331出版社
AMER CHEMICAL SOC
DOI: 10.1021/ja210270m
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资金
- National Natural Science Foundation of China [20825724]
- Shanghai Government [10dj1400100, 08GG13]
- Center for Re-Defining Photovoltaic Efficiency through Molecular-Scale Control, an Energy Frontier Research Center
- U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001085]
Described here is a new and highly general strategy for multiple-template (multitemplate) patterning. This process is significant because it allows us to create various unusual shapes such as solid spheres, yolk-shell spheres, flowerlike particles, and structured nanocomponents. Alcoholysis. of the metal-organic precursors with mixtures of glycerol and various amounts of ethanol followed by calcination yields oxides. The glycerol plays the dual role of hierarchically assembling the metal-organic composites and stabilizing the structures during the subsequent conversions. Furthermore, we demonstrate for the first time that these metal-organic composites can be converted into oxides, nitrides, and highly graphitized carbon nanostructures. We show that these yolk shell structures display superior photocatalytic activity and electrochemical properties.
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