期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 134, 期 28, 页码 11334-11337出版社
AMER CHEMICAL SOC
DOI: 10.1021/ja303220j
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资金
- National Science Foundation [CHE-0841187, CHE-1111133]
- National Institutes of Health [GM-59426]
- Direct For Mathematical & Physical Scien
- Division Of Chemistry [1111133] Funding Source: National Science Foundation
Molybdenum or tungsten monoaryloxide pyrrolide (MAP) complexes that contain OHIPT as the aryloxide (hexaisopropylterphenoxide) are effective catalysts for homocoupling of simple (E)-1,3-dienes to give (E,Z,E)-trienes in high yield and with high Z selectivities. A vinylalkylidene MAP species was shown to have the expected syn structure in an X-ray study. MAP catalysts that contain OHMT (hexamethylterphenoxide) are relatively inefficient.
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