期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 133, 期 35, 页码 13942-13945出版社
AMER CHEMICAL SOC
DOI: 10.1021/ja206580j
关键词
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资金
- Nanyang Technological University
- Singapore Ministry of Education [MOE2010-T2-1-009]
Synthetic methods for 3-azabicyclo[3.1.0] hex-2-enes and 4-carbonylpyrroles have been developed that use copper-mediated/catalyzed reactions of N-allyl/propargyl enamine carboxylates under an O-2 atmosphere and involve intramolecular cyclopropanation and carbooxygenation, respectively. These methodologies take advantage of orthogonal modes of chemical reactivity of readily available N-allyl/propargyl enamine carboxylates; the complementary pathways can be accessed by slight modification of the reaction conditions.
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