期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 133, 期 5, 页码 1168-1171出版社
AMER CHEMICAL SOC
DOI: 10.1021/ja106945v
关键词
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资金
- Ministry of Education, Culture, Sports, Sciences, and Technology
- Japan (MEXT)
- Japan Science and Technology Agency (JST)
- New Energy and Industrial Technology Development Organization (NEDO)
- Ministry of Education, Culture, Sports, Science and Technology (MEXT), Japan
We have fabricated a unique memristive device by molecular engineering and demonstrated that the leakage current tuning in the device is 100 times more efficient than that in a standard device. Molecular analogs of the memristive matrices used here are an electrochemically active conjugated Co(III) polymer (CP) and a nonconjugated Co(III) polymer (NCP), which have been synthesized in good yield and characterized by H-1 NMR spectroscopy. Redox switching of an organic-metallic hybrid polymer generates bistable states with a large ON/OFF ratio that supports random flip-flops for several hours. Thus, we provide a synthetic solution to leakage current restriction, one of the fundamental problems faced when fabricating state-of-the-art electronic devices.
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