期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 133, 期 10, 页码 3264-3267出版社
AMER CHEMICAL SOC
DOI: 10.1021/ja1102037
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资金
- JSPS [21225005]
- MEXT [22105003]
- Grants-in-Aid for Scientific Research [21225005, 22105003] Funding Source: KAKEN
Formamides having 1-arylalkyl groups on nitrogen undergo an unprecedented dehydrogenative [4 + 2] cycloaddition reaction with alkynes via nickel/AlMe3 cooperative catalysis to give highly substituted dihydropyridone derivatives in good yields. Notably, the transformation proceeds through double functionalization of C(sp(2))-H and C(sp(3))-H bonds in the formamides.
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