期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 134, 期 1, 页码 67-70出版社
AMER CHEMICAL SOC
DOI: 10.1021/ja208469n
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资金
- National Basic Research Program of China (973 Program) [2012CB821706]
- National Natural Science Foundation for Distinguished Young Scholars of China [20825102]
- National Natural Science Foundation of China [21171114, 21101103]
- Shantou University
The gyroid is ubiquitous for underlying the construction of natural substance and artificial zeolites, but it has been, surprisingly, overlooked by chemists who work in the field of metal-organic frameworks (MOFs). In this work, a series of gyroidal MOFs with gie topology, constructed from 1,2-bis((5H-imidazol-4-yl)methylene)hydrazine and octahedral metal ions, such as Zn-II, Mn-II, Cu-II, and Ni-II, have been synthesized. The Zn-II analogue, named as STU-1, shows exceptional thermal and chemical stabilities, and exhibits permanent porosity and CO2 capture ability.
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