期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 133, 期 44, 页码 17574-17577出版社
AMER CHEMICAL SOC
DOI: 10.1021/ja207180x
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资金
- Deutsche Forschungsgemeinschaft
- Alexander von Humboldt Foundation
The dinuclear lutetium dihydride dication supported by metalated tripodal ligands undergoes facile hydrogenolysis with H(2) to form a trihydride dication. Molecular orbital analysis shows that the LUMO is a bonding Lu center dot center dot center dot Lu orbital that is poised to activate dihydrogen.
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